Development of Green Colour in Topaz Using Diffusion Method

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Date
2021
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Uva Wellassa University of Sri Lanka
Abstract
Topaz is one of the abundant gem varieties in Sri Lanka with the chemical formula of Al2SiO4(F, OH)2, which has a hardness of 8 on the Moh’s hardness scale. The colourless Topaz varieties have less market value compared to the coloured Topaz varieties. Irradiation and other methods are used traditionally to improve the appearance of Topaz. Nevertheless, conventional methods have drawbacks such as high manufacturing cost, less operational safety due to radioactivity related processes. Hence, the present study tested the diffusion effect of Chromium (II) chloride on colourless topaz with the aid of heat treatment. Seventy-two colourless Topaz samples were treated with Chromium (II) chloride. The selected stones were heated under reduced and oxidizing conditions with the Chromium (II) chloride at different temperatures (600 0C, 700 0C, 800 0C, and 900 0C ) and different soaking times (1, 2, and 3 hours). In both reduced and oxidizing conditions Chromium (II) chloride, diffused into the topaz by producing a shade of pale green to dark green colour. Colour shade becomes strong with the increase of the temperature. Produced colours created a desirable appearance on the stones. At 900 0C the produced green colour was identified as ‘GB/BG 7/2’ in the GIA colour grading system. The durability of the coating was tested for acidic conditions (with HNO3 and H2SO4 acids) and sonication. The produced surface coating was stable under acidic conditions as well as under the sonication. Oxidizing conditions in electrically operated furnace is economically beneficial over gas furnace in producing colours. Finally, colourless Topaz could develop the green colour by diffusion with the optimum temperature of 900 0C with the soaking time of 1 hour under oxidizing conditions. Keywords: Diffusion Treatment; Topaz Enhancement; Colour development of gemstones
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Keywords
Mineral Sciences, Materials Sciences, Gemstones, Applied Earth Sciences, Geochemistry
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